-31- large plankton and Mo?9--T.29™ were higher in small plankton; otherwise the radioisotopic compositions were similar. Analysis of sea water collected shortly after another underwater detonation (Umbrella), in the lagoon at Eniwetok, showed that Np pel32_82 Ce!43_ pr l43 and Mo?9-p¢99m were 239 ’ the predominant radioisotopes in the particulate matter (>0.45u) present in the surface water near target zero (Table 8). Table 8. Percentage of gamma emitting radioisotopes in the particulate (> 0.454) and soluble (<0. 45y) form in sea water collected 75 minutes after the Umbrella event (8) Radioisotope Particulate 108 d/m/1 Per cent of particulate activity Soluble Per cent of soluble 106 d/m/1 activity Np239 5.2 62.5 30.0 75.6 y237 0.02 0.2 4.0 10.1 Tel32_1132 1.9 22.3 1.9 4.7 Mo29-T¢99m 0. 48 5.8 3.1 7.8 Cel4l-pyl4l 0.028 0.3 0 Cel43-pyl43 0.66 7.9 0 Cel44.py144 0. 0028 £0.14 0 Bal40_1,4140 0.076 Some of these isotopes also the <0.45yu fraction (Table 8), 0.9 were present which could 0.7 in high 1.8 amounts in include materials

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