UNCLASSIFIED
When separating trace quantities from an interfering bulk electroayte, the predominant problem usually involves the effect of co=precivitation of the bulk electrolyte or its incompleteness of sepa

ration.

Likewise in radio-assay work, the weight of the bulk elect

brought down with the carrier added as part of the procedure can le
to low recoveries, mainly by self-absorption of the emitted particl
by the sample during counting.

Ow

Figure A=3 shows the effect of increasing amounts of strontium carrier
upon the activity. Non=strontium impurities would show the seme
effect if they are carried down with the strontium nitrate precipitate since the major impurity is calcium, it is best to know the

solubility of Ca(NO3)2 in 75% HNO, so as to insure completeness of

removal.

This was found to be equivalent to 23.5 grams of CaO per

liter of the 75% acids

Concentrations above 75% HNOs markedly re-

duce the calcium solubility, while cormentrations below may cause

too great a solubility loss of strontium, as shown in the factorial
reported.
An experiment was performed to determine the effect of calcium on
the recovery of Sr®°, Solubility measurements indicated that 200 ml]

of 75% HNO. would cause a loss of 2.6 mg of Sr or a 13% loss when

using 20 mg Sr carrier.

Table A=) indicates that the presence of

calcium does have a salting effect and that the Sr recovery will be
improved by operating close to calcium saturation. If no calcium

is present, then a minimum of HNO, should be used.

% Saturation

1.

2.

3.
he

100 (4.7 g Cad)
75

50
25

c/r

& Recovery

1880

91.3

1855
1815

90.0
83.0

1895

91.9

The chemical separation involved in the isolation of Sr®* or y*°
from varicus samples may be subject to interference from cther

fission products.

Table A=5 lists elements mich combine possitle

chemical interference with long nelf-life. Their characteristics,
along with the perentape of total fission prodyect activity wnich
they represent at various times efter detonation, are given in the
table along with the corresvonding properties for the strontium anc
yttriun fission products.

wre SRE
UNCLASSIFIED

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