~3— Pasurements of samie-rey enlisting Pission proguces have ves aoe a made periodically on soils sollected at tha irgorne National Laboratory site siswe the spring of 1957. Tho measuring teehniara orvloyed was that of gamma-ray apectromstry of soll samples of finite wise (1-2 zg} : using a 5° by 4° Nal eryeteal and en aygonne Pyve 256 channel analyser. The soil was geometrically arranged by means of a steimiess obesl eontainer into a one inch layer sromd and over the exyatal (6). Beckground reduction, essential for the detection of the quantities rm , 7 sample and dstector. & + ce 2 3 3 was effected througn the uss of thick stesl shieldiag az iferry of achivity involved (approximately 10”10 ouris of os?! fkg of soil), Soil sampling was dons to a depth of 6 inehes go thet essentially all fission products present over a given aren yers inciuded. Two gamma-ray spectra of soll taken with en Ral erystal are shown in Figure 2, The one from deep soil is free of sny fission activity end contains only Th, 0, ane °°. The other, from soil collected in July 1959, indicates the sresence cf two peaks not eyident in the first case. Tha one seal is due to Beoily9 and the other to Ru} ,106, The concentration of fission and natural radicactivity in soit was de determined by the use of sources cf tmown acbiviby imeorperated in moek soil (HagFO4) > The wethed presupposss imovledes of the varions isotopes present in the soil, The stenderd reference spectra, ome for each isotope, permit setting up the fraction of the total counting rate oceurting in orxch spostrel region, there being ea many regions 238 Los e Te MB RCH EES

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