isotopes in appreciable amounts. Detailed studies were undertaken to establish with certainty the identity of the isotopes and to determine their contribution to the total activity in the Rongelap soil. ’ MATERIALS AND METHODS A 1.68-gram portion of soil ash, equivalent to 18.1 grams of dry soil, taken from the top inch in a bird nesting area at Kabelle Island on July 18, 1957, was dissolved in 0.2 N HCl and passed through an ion-exchange column to separate the radioisotopes present in the sample. (The method used was described in detail by Lowman, Palumbo, and South). 14 For this.experiment a cationic resin (Dowex 50*) of 50- 100 mesh and columnsize of 0.942 cm@ x 61 cm was used. The sample and the eluting agents were passed through the column ata flow rate of one ml/min. A summary of the volumes used and the radioisotopes eluted is given in Table 1. Aliquots of the fractions collected were counted for beta and gammaactivity, and those fractions with significant amounts of gamma radioactivity were analyzed in a single-channel, 50-position, automatic-advance, gamma spectrometer 1 well-type sodium iodide crystal. 7 * Available from Dow Chemical Co., Midland, Michigan with a 2-inch,

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