(Reprinted from Nature, Vol. 202, No. 4934, pp. 745-749, May 23, 1964) SPECTROMETRIC DETERMINATION OF DOSE RATES FROM NATURAL AND FALL-OUT GAMMA-RADIATION IN THE UNITED STATES, 1962-63 By WAYNE M. LOWDER, HAROLD L. BECK and WILLIAM J. CONDON Health and Safety Laboratory, U.S. Atomic Energy Commission, New York ” [THE Health and Safety Laboratory of the U.S. Atomic Energy Commission has boen examining for nearly a decade the dosimetric properties of environmental radiation, particularly the natural components. Instrumentation and analytical techniques have been developed which are directed toward securing preciso interpretations of in situ radiation measurements in terms of air dose rate!-3, from which quantities of biological interest may be derived. Because of the importance of total body and genetic exposure in considerations of the long-term interaction between ionizing radiation and man, our interest has been focused on the more penetrating radiations. These include tho y-radiation from potassium-40 and the daughters of radium-226 and thorium-232 in the arth and the ionizing component of the cosmic radiation, consisting primarily of the high-energy muons and electrons. We have also had to take account of the presence of fall-out in the environment, and havo devel- oped techniques for determining the individual dose-rate contributions to the total environmental y-field of the various significant natural and fall-out y-emitters. These techniques are described in this article and a summary of the field data obtained during 1962 and 1963 is given. During the late 1950’s, the importance of the y-radiation from locally deposited fission products from weapons tests was first noted. Gamma dose rates considerably in excess of the ambient natural levels were recorded by a number of investigators either by direct monitoring*‘-* or by inference from soil and/or air sample analyses?-!°. Similar increases were noted during the testing period that began in September 1961 (refs. 11-14). Under such conditions, ionization chambers have proved valuable as monitors of changes in total environmental radiationlevels at individual locations, particularly when the mean natural radiation-levels are known from readings taken during periods of little or no fall-out‘-*!4. Other techniques are needed if such readings are not available or if it is desired to survey newlocations.

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