Our ionization chamber measurements at several of the lake sites were quite consistent with simultaneous measurements by the NYU group although they do appear to be slightly lower at the higher altitudes.” This may be due to the effect on our thicker-walled chambers of a slight change in the cosmic ray secondary energy spectrum with altitude. Spectrometric Determination of 137¢s Concentrations in Soils Spectrometric number of U. sites. S. measurements were made at or near a Department of Agriculture - HASL soil samplinc Estimates of the total activity of 137cs present in the soil at these locations were made from the 13’cs dose rates determined by our spectrometric techniques.* These estimates will be compared with radiochemical determinations of 137cs and 90Sr in recent soil samples taken at these sites in order to determine the validity of applying our field spectrometric technigues to study fallout deposition. We assume fallout to be distributed with depth in the soil according to the relationship S = So e-2/4 where S (mc/cn is the activity at depth z (cm) below the surface and So is the activity at the surface.* We routinely use a relaxation length a = 3 cm and an in situ density of 1.6 gm/em3 (average over top 6" of soil) to represent a typical situation. The flux and total dose rate from such an exponential distributior depend on the quantity ap, where p is the density.® For a given a and p the dose rate at one meter above the ground per 100 mc/mi? of activity can be calculated as can the expected number of 0.66 Mev 137’cs absorption peak counts for our detector per unit dose rate and the expected number of counts per 100 mc/mi2 total soil activity. In order to illustrate the magnitude of the error involved in determining the 137¢s dose rate and soil activity from a spectrum for a particular site the values of the above guantities are given below for 4 different products of a and p

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