SESSION HIB DISCUSSION 697 HAWLEY: Dr. Libby has suggested that there may be a selective plant-uptake mechanism involved in the transpiration of tritiated water over normal water. This, if true, may help explain such things as the greater concentrations of 3H over continents than over oceans and over large forested areas than over semiarid areas and also seasonal variations. Dr. Thatcher, has your group been considering this? THATCHER: By analogy with deuterium, one might expect that a selective plant-uptake mechanism with respect to tritium might exist. The plant would reject tritium as it usually does deuterium in the metabolic process, and this would increase the evaporation of tritiated water leading to a higher air concentration. The IAEA data do not appear to support this mechanism, however, since the concentrations found in semiarid regions, such as at Teheran, are generally just as high as those in regions that support an abundant vegeta- tion, such as at Vienna. The more humid regions are more greatly influenced by oceanic air, however, which would counteract the pro- posed effect for vegetation. The data should be carefully scanned in an attempt to identify this effect. BOLIN: There is, of course, fractionation when evapotranspiration takes place from vegetation. It is important to realize, however, that, for estimating this, the effect of water transfer through the capillary systems in the plants must be considered. We do not know precisely what the final effect is, but changes in the composition of water due to fractionation insofar as tritium is concerned is small compared to the variations that have been observed in precipitation. REITER: Dr. Bolin, did you imply that from tritium measure- ments at the ground, together with knowledge of the observed tritium gradient in the atmosphere, you could make inferences on the precipitation physics in the atmosphere? BOLIN: The vertical transfer of tritium, deuterium, ‘80, and particulate matter takes place through the same mechanism of turbu- lence. Since the sources and sinks of these tracers are different but partially related, observations of the vertical distribution of all of them would yield some information on the turbulent processes and the intensity of the transfer. Considering the vertical distribution in the trade-wind belt to be in an approximate steady state might yield information on the turbulent transfer of water vapor and have a bearing on our estimates of evaporation from the ocean surface. I am not sure how such data would be precisely interpreted, but in any case the simultaneous use of several tracers for studies of the vertical transfer should be advantageous.

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