GLOBAL DISTRIBUTION OF TRITIUM The 667 increase of tritium concentration toward the northern mid- latitudes is clear. Southern-hemisphere tritium data for the Pacific is represented by Canton Island (LJ) and Kaitoke, New Zealand (NZ) (Figs. 2 and 7). Canton at 02°46’S shows typical southern-hemisphere values for 1963, averaging 9.4 T.U. At Kaitoke the mean tritium concentration for the same period is 24.2 T.U. There is no evidence of a peak at Canton, but a spring peak is clearly defined at Kaitoke. Although Kaitoke may be influenced by the land mass of New Zealand to some extent, this effect would not appear to be very Significant because of the overwhelming ratio of water over land area. Kaitoke is a coastal location (near Wellington). Thus it appears that the higher mean concentrations at Kaitoke may represent a true latitude effect. This would suggest the entry of the annual tritium fallout pulse at the higher southern latitudes and gradual migration of the pulse northward. The Americas The highest tritium concentrations in the entire survey with the single exception of Nord, Greenland, are found in northern Canada (Fig. 8). Although the 1961-1962 record for Canada is not complete, it seems fairly certain that these northern sites showed the same im- mediate response to the Oct. 23 to 30, 1961, testing that was observed in the Arctic regions of Europe. In January 1962, for example, the tritium measurement at Whitehorse, Yukon (CR), was 1010 T.U., and at Goose Bay, Labrador (CR), it was 1680 T.U. The single highest monthly tritium measurement found throughout the entire survey was the 10,000 T.U. value for April 1963 at Whitehorse. The effect of the prevailing cross-continent direction of air circulation may be observed in Canada where west and east stations are located at approximately the same latitude. The difference is most marked in 1961 when the influx of spring tritium was minimum (com- pared to later years) and reevaporated tritium showed its maximum effect. Between Edmonton (53°34’N, 113°31'W) and Goose Bay (53°19'N, 60°25 W), an apparent time difference of approximately one month existed between the fall tritium decay curves, with the summer peak persisting longer at Goose Bay. This was as expected. The same effect is not observed in 1963 for Edmonton and Goose Bay, but it is suggested for Whitehorse and Goose Bay. Presumably, as the proportionate input of stratospheric tritium decreases and the reevaporation component increases, in 1964 and 1965 the delay of the annual tritium decline in the east as compared to the west should reappear.

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