PARTICLE ANALYSIS PROGRAM AT LAWRENCE RADIATION LABORATORY ROBERT E. HEFT and JAMES S. KAHN _ Lawrence Radiation Laboratory, Livermore, California ABSTRACT A program has been established for determining the distribution of individual radionuclides in particulate radioactive material. Particulate samples collected at their point of origin and selected on the basis of the degree to which they represent the true particle population are separated into groups and analyzed on a totality basis. The overall analytical program is described, and an example is given of the initial information produced in a particle-group separation performed on a filter sample from the Sedan shot. INTRODUCTION The Particle Analysis Program at the Lawrence Radiation Labo- ratory (LRL) is concerned with characterizing particulate radioactive material as a function of sedimentation rate. Particulate samples collected at their sources are separated in the laboratory into fractions corresponding to discrete sedimentation-rate intervals. Each fraction is then subjected to chemical, physical, and radioisotopic analyses to. provide a complete inventory, according to particle class, of each radionuclide studied. In addition, chemical composition, size distribution, density, and crystallographic character of the particles are determined for each fraction. The data provided by this program are directly applicable to three main problem areas: fallout, particle formation, and biological availability. 150

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