~ 20 = The differential rates at which the fallo - has been occurring probably are best measured by the so-call: 2 "pot collection" method. A bucket with vertical wails o: appreci- able height is placed out in the open and allowed to collect the total fallout for a given period including the rain, snow, dust, etc, The bucket is left out whether it has rained or not and covers the total fallout for a given period. Figures 6 and 7 give the curves so obtained for New York and Pittsburgh areas together with the estimated errors of measurement. It is interesting to note the changes in slope and to correlate them with the occurrence of test activities and the relatively short-lived tropospheric fallout. The minimum slopes which appear during quiet periods when no one is testing are the stratospheric fallout of which we heave spoken and these Slopes when we have enough pots operating all over the world will, when taken together with the results of the measure» ments of the amounts of radiostrontium and radiocesium in the.stratosphere, give an accurate value fer the stratospheric residence time and settle the mixing question. In addition to the intensity of fallout, the ques-~ tion of the fraction of the radiostrontiwa, and, fer tropospheric falicut, the radioiodine of sight-day half-life, that is in assimilable form is an important one. So far most fallout strontiyun appears to be completely water soluble and therefore most assimilable, though continued tests cn this point should be made. Direct leaf pick-up of course promotes assimilation of the strontium because the plant differentiation against strontium when it assimilates it from soil thus is avoided. Another factor is, of course, the concentration of available calcium in the sozrl. By szvailable calcium we mean calcium which is available to rlants and not che tetal calcium in the soil. I% is known that soils which are high in available calcium produce plants cf lower radioactive strontium content; that is, the radicactive strontium to calcium ratio in the plant is lower as a direst consequence of the lower concentration of radiostrontium in the available soil caiciun. In addition, as mentioned previously, plants tend to prefer calcium to strontium with a discrimination facter of about 1.4. Sheep which grow in certain areas of Wales have shown concentrations in their bones approaching 150 Sunshine Units, while sheep and cattle growing in the U. S. have hardly ever exceeded one-fifth of this. The Welsh soil in certain areas oD ee et be FF « © i £F . «© 4 £ 1 &€ ” EB ™ ra (more)

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