After the initial gross activity was surveyed, samples of humanhair, grass, thatch roofing, and soil were analyzed for their beta and alpha activity (Table 4.9). The presence of fissile material on the thatch was of the order of 107° ng/g and on grass about one-half that on the thatch, at 35 days postdetonation. The fissile material activity in human hair was quite low. TABLE 4,9—-Gross Beta and Alpha Activity of Soil, Grass, and Thatch from Rongelap Days Sample post- detonation Beta activity (Sr® equivalent) pe/e Fissile material (ue/g * 10°) Thatch T1-5 T6 35 56 2.7 1.6 1.3 35 0.5 0.3 67 67 0.09 0.03 S1 (organic) 41 0.10 0.47 $3 (surface) 67 0.06 3.0 Grass G1-3 G4 G5 G6 (Utirik) 41 0.3 0.1 Soil 82 (sandy) 4.3 41 0.06 S4 (6 in. deep) 67 0.003 85 (Utirik) 87 0.006 0.03 1.9 0.8 SUMMARY AND CONCLUSIONS The fallout material was found to consist largely of calcium oxide and calcium carbonate. The fission products were adsorbed mainly on particles of 60 to 200 up. This material was 10 per cent soluble in water and completely soluble in acid. Radioanalysis of soil and water samples from Rongelap indicated high levels of radioactive contamination from the fallout at early times following detonation. Significant amounts of beta activity as well as smaller amountsof fissile material were present on the external surfaces of plants 42 days after detonation. Only small amounts of beta activity and no alpha activity were detected in the edible portion of foods. It appears that during the first month a limited amount of fission products is available to plants growing on contaminated soil. However, high levels of activity in the coconut tree sap were detected which had an isotopic composition very similar to that of the water analyzed. Radiochemical analysis of thatch and water samples indicated a marked variation in the ratio of Sr®, Ba‘“°, and the rare-earth group probably as a function of the different solubilities of the radioelements. The activity of food, water, and soil samples from Utirik was approximately Yh of those of Rongelap. It appears from this study that the ingestion of contaminated water was oneof the principal sources of contamination for the Marshallese. Of the individual radionuclides, Sr®*, because of its high solubility and relatively long half life, was probably the isotope of greatest potential hazard in the environment. 47

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