A
n
i=n
i=]
=f
j=n-1
jen
nods fey, 5
jai
Jed"
js;
a2 Ast
DOU
pan
To
pi
pF j
(4)
Oy -X;)
where
i
roy
~
A, = the number of atoms of the nth member of an isobaric chain at time
t post detonation per unit fission,
the independent yield at t = 0 of the it" isobar in the A,
a
>»
isobaric chain per unit fission,
j
decay constant of the zth isobar,
£5, j+1 = branching fraction of the gth isobar leading to the
creation of the yth + 1 isobar,
t ™ time post BRAVO detonation.
The use of Eqs. 3 and 4 led to the inclusion in Table 5 of all
fission products with the exclusion of only a few of the dosimetrically insignif-~
icant ones.
A few important transuranics and activation products were included
in Table 5 based on the Tsuzuki measurements on day 26 fallout (Ts55) and use of
parent-daughter transformation equations given by Bateman (Bal0).
d.
Non-Fission Fragment Nuclides Not Accounted For
The nuclides which may have been present at some level but re-
main unaccounted for are Be-7, Na-24, Mn-56, Fe~55, Fe-59, Co-57, Co~58, Co-60,
Cu-64, Cu~67, U-240, Np240m, Np-240, Am-241 and Cm-242.
Two short lived activa-
tion products, Na-24 and Mn-56, might have accounted for some of the exposure
rate measured at day 2.2 at Rongelap Island.
Borg (Du56) tabulated the photon
energy spectrum from a BRAVO fallout sample collected at Rongelap Island.
fallout sample was reported to be analyzed at 4 days post detonation.
trum showed a significant peak energy at 850 keV.
The
The spec-
Mn-56 has a characteristic
photon at 847 keV but so do about 30 other nuclides that were present in fallout
at that time (RSIC73).
Mather (Du56) indicated that short-lived neutron activa19