Project Title:

16.

Molecular and Cellular Radiobiology

Storage and Transfer of the Genetic Message
Technical Progress in FY 1973: (Cont'd.)

RX-03-02-(d)

However, this work with ethidium bromide did not follow the change in
layer-line spacing with increasing bound drug; the value was based on

molecular model-building,

Although two other papers have described x-ray

diffraction studies of the intercalation of planar molecules with DNA, a
key contribution from the studies reported here on the interaction of

daunomycin with DNA was the location of the first zero in the equatorial
Fourier transform, described for the first time in such interactions.

This

gave hard evidence on the molecular geometry of the complex,
The value
derived in these studies for the untwisting of the DNA helix per molecule
drug bound is most important in studies on circular DNA and will become

increasingly important in studies on the structure of the chromosome and how

the chromosome functions,

™

‘

All previous evidence suggesting that daunomycin intercalates into
DNA was based on solution studies whose interpretation rests on analogies
with similar studies on ethidium bromide and the acridines.
For these
molecules earlier x-ray work was taken as major evidence for intercalation;

but, in fact, it was not nearly so unambiguous as the x-ray data reported in

these studies on daunomycin and DNA,
In sum this is a contribution to the
stereochemistry of intercalation, widely assumed to be a key mechanism in
the action of many basic drugs and a possibly important way in which polynuclear hydrocarbons, largely emitted by the burning of coal, interact with

the informational macromolecules to induce such late effects as oncogenesis.

:

The single crystal analysis of the 1:2 complex of actinomycin with
deoxyguanosine by Sobell and collaborators provides strong evidence for

an intercalation model for the interaction of actinomycin with the DNA
double helix.
An earlier model proposed by Hamilton, Fuller, and Reich
was based on specific hydrogen bonding between groups on the actinomycin

with those on the guanosine residues in the DNA, Ome difficulty with the
intercalation model is that the basis for the high specificity of the
DNA-actinomycin interaction is not clear,
It may be, therefore, that the

external binding model represents a transient recognition state which is a
preliminary to strong binding of the actinomycin through intercalation,
In fact, for many molecules which bind to DNA, there appears to be an
equilibrium between a strong intercalation binding site and a weak external

binding site, Work here on daunomycin binding showed that the degree of
intercalation varied with the relative humidity of the environment in which
the
rs of the DNA daunomycin complex were maintained.
The degree of
int
beca

faction increased with the increasing relative humidity presumably
increase in the amount of water in the fiber environment tended
a~the

to increase the hydrophobic contribution to the intercalation interaction,
Experiments to date with DNA-actinomycin fibers have not yet given clear
evidence for intercalation.
However, these studies are being extended by
maintaining fibers of the complex at very high humidity in an effort to
favor the intercalation type of binding.

(See Continuation Sheet)

pi vazis

RX-254

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