Health Physics Pergamon Press 1978. Vol. 34(March), pp. 209-217. Printed in Great Britain

407958

ANALYSIS OF ALPHA EMITTERS IN
THE CORAL, FAVITES VIRENS,
FROM BIKINI LAGOON BY SOLID-STATE
TRACK DETECTION
YITZHAK LEVY, DONALD S. MILLER and GERALD M. FRIEDMAN

Department of Geology, Rensselaer Polytechnic Institute Troy, NY 12181
and
VICTOR E. NOSHKIN

Lawrence Livermore Laboratory, Livermore, CA 94550
(Received 8 November 1976; accepted 10 July 1977)
Abstract—A quantitative method for the non-destructive analysis of alpha emitters in
CaCO, matrices by solid-state track detection (cellulose nitrate) was developed.
0.4 pCi/g in an area of 4mm7?can be measured routinely; smaller concentrations can
be determined but with a lower resolution. Calibration methods used were (a) a Pu source
of 0.15 wCi in conjunction with polycarbonate and CaCO, absorbers of different thickness
(2-30 um) and (b) a powdered coral sample from Enewetak Atoll which had been
tadiochemically analyzed for plutonium radionuclides, **'Am and other long-lived fission
and activation products.
Slabs of a coral, Favites virens, from Bikini lagoon were analyzed. A quantity of the
alpha emitters detected in regions of the coral identified with growth during the years of
nuclear testing (1954, 1956 and 1959) are found in small discrete spots. Thin sections cut
parallel to the direction of coral growth give different patterns of distributions. No such
“hot spots” are evident in any post-test year growth sections although plutonium and
other long lived fission and activation products were measured in these sections by
radiochemical techniques.

INTRODUCTION

Many applications of solid-state track detectors have been made in several fields of
engineering and science (F175). Alpha-particle
detection using cellulose nitrate as the solidstate track detector has been developed to
the stage whereby distribution of alpha emitters at very low concentration levels can be
determined. The efficiency for the solid-state
alpha track detector (Kodak LR-115, Type I)

was determined using a very thin 7’Pu cali-

brated source in conjunction with alpha
energy degraders of polycarbonate and calcium carbonate films and a powdered coral
sample of known plutonium and americium
activities.

A coral, Favites virens, collected alive from
Bikint lagoon in 1972 was sectioned for
analysis. Relatively high radionuclide levels,

including plutonium radionuclides and “'Am,

were detected in the coral growth sections
corresponding to the nuclear testing years of
1954, 1956 and 1958 (No75). Since it has been

demonstrated (Ba74) that coral skeletons are

excellent samplers for suspended particulate
material in the water column it was of interest to determine whether the radionuclides
detected in the coral-growth increments were
taken up as dissolved species or were taken
up, in part, through particulate incorporation.
Through the application of the solid-state

alpha detector to slabs (1 cm thick) and thin
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